Diabolical points in the magnetic spectrum of Fe_8 molecules

The magnetic molecule Fe_8 has been predicted and observed to have a rich pattern of degeneracies in its spectrum as an external magnetic field is varied. These degeneracies have now been recognized to be diabolical points. This paper analyzes the diabolicity and all essential properties of this system using elementary perturbation theory. A variety of arguments is gievn to suggest that an earlier semiclassical result for a subset of these points may be exactly true for arbitrary spinComment: uses europhys.sty package; 3 embedded ps figure

Instanton picture of the spin tunneling in the Lipkin model

A consistent theory of the ground state energy and its splitting due to the process of tunneling for the Lipkin model is presented. For the functional integral in terms of the spin coherent states for the partition function of the model we accurately calculate the trivial and the instanton saddle point contributions. We show that such calculation has to be perfomed very accurately taking into account the discrete nature of the functional integral. Such accurate consideration leads to finite corrections to a naive continous consideration. We present comparison with numerical calculation of the ground state energy and the tunneling splitting and with the results obtained by the quasiclassical method and get excellent agreement.Comment: REVTEX, 32 pages, 3 figure

Statistical mechanics of temporal association in neural networks with transmission delays

We study the representation of static patterns and temporal sequences in neural networks with signal delays and a stochastic parallel dynamics. For a wide class of delay distributions, the asymptotic network behavior can be described by a generalized Gibbs distribution, generated by a novel Lyapunov functional for the determination dynamics. We extend techniques of equilibrium statistical mechanics so as to deal with time-dependent phenomena, derive analytic results for both retrieval quality and storage capacity, and compare them with numerical simulations

Oscillatory Tunnel Splittings in Spin Systems: A Discrete Wentzel-Kramers-Brillouin Approach

Certain spin Hamiltonians that give rise to tunnel splittings that are viewed in terms of interfering instanton trajectories, are restudied using a discrete WKB method, that is more elementary, and also yields wavefunctions and preexponential factors for the splittings. A novel turning point inside the classically forbidden region is analysed, and a general formula is obtained for the splittings. The result is appled to the \Fe8 system. A previous result for the oscillation of the ground state splitting with external magnetic field is extended to higher levels.Comment: RevTex, one ps figur

On the Observability of Meso- and Macro-scopic Quantum Coherence of Domain Walls in Magnetic Insulators

Results are presented of a numerical calculation of the tunneling gap for a domain wall moving in the double well potential of a pair of voids in a magnetic insulator. Both symmetric and asymmetric double well potentials are considered. It is found that, even in the absence of dissipation, the prospects for observing quantum coherence on a meso- or macro-scopic scale appears unlikely.Comment: 15 pages, Plain LaTex, UBC TP-93-1

Quantum phase interference and spin parity in Mn12 single-molecule magnets

Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the magnetic field applied along the hard anisotropy axis are due to topological quantum phase interference of two tunnel paths of opposite windings. Spin-parity dependent tunneling is established by comparing the quantum phase interference of integer and half-integer spin systems.Comment: 5 pages, 5 figure

Strong Coupling Theory of Two Level Atoms in Periodic Fields

We present a new convergent strong coupling expansion for two-level atoms in external periodic fields, free of secular terms. As a first application, we show that the coherent destruction of tunnelling is a third-order effect. We also present an exact treatment of the high-frequency region, and compare it with the theory of averaging. The qualitative frequency spectrum of the transition probability amplitude contains an effective Rabi frequency.Comment: 4 pages with 3 figure